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Ratnasamy P, Raja R, Srinivas D: Novel, benign, solid catalysts for the oxidation of hydrocarbons. Philos Transact A Math Phys Eng Sci. 2005 Apr 15;363(1829):1001-12.
Monomeric copper phthalocyanine and salen complexes entrapped in zeolite-Y oxidize methane to methanol, toluene to cresols, naphthalene to naphthols, xylene to xylenols and phenol to diphenols.
In almost all cases, the intrinsic catalytic activity (turnover frequency) of the metal complex is enhanced very significantly, upon encapsulation in the porous solids. |
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